Pivotal Role of Cloud‐Planetary Boundary Layer Coupling to Explain Contrasting Aerosol‐Cloud Relationships
The radiative effect of aerosol on cloud albedo via altering cloud droplet effective radius (re) is a major uncertainty in the Earth's climate system. Remote sensing studies have reported either negative or positive relationships between re and aerosol number concentration (Na) or other aerosol proxies. However, there are much fewer in situ observational evidences and physical explanation remains elusive for the contrasting Na-re relationships. Here we quantify the Na-re relationship by using in situ aircraft measurements, together with a re decomposition method. Our analysis reveals that the cloud-planetary boundary layer (PBL) coupling plays a pivotal role on the Na-re relationship.more »